Redox Potentials and Electronic States of Iron Porphyrin Ⅸ Adsorbed on Single Crystal Gold Electrode

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  Metalloporphynns are active sites in metalloproteins and synthetic catalysts.[1]We recently used iron protoporphyrin Ⅸ(FePPⅨ) as an intercalating probe for long-range electrochemical electron transfer through a G-quadruplex oligonucleotide(DNA-zyme);this study disclosed two,rather than a single pair of voltammetry peaks with a new and dominating peak,shifted 200mV positive to the ≈-0.4V peak.
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