Theoretically and experimentally, folds and wrinkles are unavoidable to be induced in graphene whatever graphene is prepared by micromechanical exfoliation from graphite or chemical vapor deposition.Many advantages developed by graphene wrinkles have been realized such as great improvement of stretchability of graphene and utilized flexible electronic devices and energy storage.However,controllable fabrication of wrinkled graphene is still a big challenge for its applications.Here, we report a facile liquid-phase shrink method to controllably fabricate large-scale wrinkled graphene with nanoscale wrinkles.As-prepared samples with macroscopically rectangular shape and homogeneous wrinkled structures are characterized using optical microscopy, scanning electron microscopy (SEM),transmission electron microscopy (TEM), atomic force microscopy (AFM), Raman spectra and mappings.Transmittance and sheet resistance measurements of the samples were performed to exhibit the excellent optical and electronic properties respectively.