Sol-gel derived oxides and mixed oxides catalysts with narrow mesoporous distribution

来源 :Science in China(Series B) | 被引量 : 0次 | 上传用户:ktaxx01
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A novel sol-gel process for preparing oxides and mixed oxides sols from precipitation and peptization process is reported in this article. Inorganic salts are used as raw materials in this study. It is found that the amount of acid has great influence on the stability and particle diameter distribution of the precursor sols. Ultrasonic treatment is used to prepare alumina sol at room temperature. The result of 27AI NMR shows that there exist AI_13~(7+) species in the sol. By controlling the sol particles with narrow particle diameter distribution, alumina, titania and silica-alumina (SA) materials with narrow mesoporous distribution are formed by regular packing of sol particles during gelation without using any templates. The results also show that the structure and particle diameter distribution of precursor sol determine the final materials’ texture. A novel sol-gel process for preparing oxides and mixed oxides sols from precipitation and peptization process is reported in this article. It is found that the amount of acid has great influence on the stability and The result of 27 AI NMR shows that there exists AI_13 ~ (7+) species in the sol. By controlling the sol particles with narrow particle diameter distribution , alumina, titania and silica-alumina (SA) materials with narrow mesoporous distribution are formed by regular packing of sol particles during gelation without using any templates. The results also show that the structure and particle diameter distribution of precursor sol determine the final materials’ texture.
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