Researches on chemically modified electrode V.Catalytic reduction of oxygen on iron porphyrin modifi

来源 :Acta Chimica Sinica(English Edition) | 被引量 : 0次 | 上传用户:redmend
下载到本地 , 更方便阅读
声明 : 本文档内容版权归属内容提供方 , 如果您对本文有版权争议 , 可与客服联系进行内容授权或下架
论文部分内容阅读
By surface organic synthesis a Fe(Ⅲ)tetra-o-aminophenyl porphyrin modified electrodewas successfully prepared on glassy carbon electrode surface through amidization.The preparativeconditions were investigated in detail.Using cyclic voltammetry and semidifferential neo-polarogra-phy in an acidic aqueous solution the behavior of the catalytic reduction ofoxygen on iron porphyriamodified electrode was studied.Based on experimental results it was shown that the irreversibleprocess of 2-electron-reduction to hydrogen peroxide belongs to EC parallel catalytic process. By surface organic synthesis a Fe (III) tetra-o-aminophenyl porphyrin modified electrodewas successfully prepared on glassy carbon electrode surface through amidization.The preparativeconditions were investigated in detail. Using cyclic voltammetry and semidifferential neo-polarogra-phy in an acidic aqueous solution the behavior of the catalytic reduction ofoxygen on iron porphyriamodified electrode was studied. Based on experimental results it was shown that the irreversible process of 2-electron-reduction to hydrogen peroxide belongs to EC parallel catalytic process.
其他文献
近几年来,国际排联为了解决世界排球运动发展中的两大难题--进玫强于防守和比赛时间难以控制,对竞赛规则作了走马灯似的修改,以提高比赛观赏性和适应商业利益的需要。1999年起实
黑方刘昌赫白方李昌镐(1998年2月5日弈于韩国釜山)李昌镐是公认的“天下无敌”棋手,也是第一届LG杯世界棋王的获得者。李昌镐在1997年的比赛中胜率高达83%,令世界所有棋手瞠目结舌。在他17%的输棋中
The title compound(6),a new derivative of coumarin,has been synthesized.The overallyield,using esculetin(1)as starting material,was 3.7%.The stereochemistry of
一、引言传统的渗碳方法,都是在高温下(Ac_3以上)提高钢表面γ相固溶体的碳浓度,从而在随后的淬火中使表面层成为高硬度的马氏体。其表面碳浓度通常控制在0.8-1.0%C的范围,
碳纤维复合材料与环氧树酯复合是六十年代出现的一种新型材料,具有较高的比强度和比钢度(比重均为1.6克/厘米~3),比玻璃钢还轻,以及有好的化学稳定性,耐酸、耐碱、耐油等优
去年读钟耕略君寄自纽约的通讯,才知道有一部名叫《光之梦》的电影记录画家洛佩兹·加尔西亚的创作生活。我曾为此访求录相带未果。昨日忽见系里姜君弄到了这个录相带,喜出望外
描写边防军人生活的戏剧作品已 经很多了,但看了总政话剧团演出的话剧《老兵骆驼》(编剧孟冰,导演汪遵喜)我仍然感动不已。然而,这感动不是来自剧中人物的高大形象和丰功伟绩,
In this paper,the construction of M-band semi-orthogonal wavelets and some examples of B-spline wavelets are given. In this paper, the construction of M-band s
中国传统戏曲历史悠久,剧种繁多,是我们中国的传统戏剧。传统戏曲过去表现的多是帝王将相,才子佳人等历史题材的传统剧目,随着时代的发展,我们的传统戏曲在保留部分优秀的传
海南吊罗山热带山地雨林扫把青冈+鸭脚木群落共出现44个科,95个属的乔木树种190种,其中种类数量大于5个的有樟科(24种),茜草科(17种),山毛榉科(17种),山矾科(11种)和山茶科(1