Stabilization effects of third element on CaCu_5 type derivatives of rare-earth transition-metal int

来源 :Progress in Natural Science | 被引量 : 0次 | 上传用户:whb35750
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Part of the results of the key project “Search for novel rare-earth functional materials” supported by the National Natural Science Foundation of China is reviewed. In combination with reports in literature, the effects of the third element M on the formation and stability of La2(Co, M)17, R(Fe, M)12 and R3(Fe, M)29 intermetallic compounds are discussed by considering mixing enthalpy of M with rare-earth, Fe and Co, and atomic radius, electronegativity and electronic configurations, etc. It is concluded that the mixing enthalpy and atomic radius dominate the preferential sites and the minimum amount of M required to stabilize a structure, which ultimately affect the magnetic properties of a compound prominently. This review should provide some heuristic hints for exploiting novel rare-earth transition metal functional materials and for improving their performance. Part of the results of the key project “Search for novel rare-earth functional materials ” supported by the National Natural Science Foundation of China is reviewed. In combination with reports in literature, the effects of the third element M on the formation and Stability of La2 (Co, M) 17, R (Fe, M) 12 and R3 (Fe, M) 29 intermetallic compounds are discussed by considering mixing enthalpy of M with rare earth, Fe and Co, and atomic radius, electronegativity and electronic configurations, etc. It is concluded that the mixing enthalpy and atomic radius dominate the preferential sites and the minimum amount of M required to stabilize a structure, which ultimately affect the magnetic properties of a compound prominently. This review should provide some heuristic hints for exploiting novel rare-earth transition metal functional materials and for improving their performance.
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