Nanofibrils in 3D aligned channel arrays with synergistic effect of Ag/NPs for rapid and highly effi

来源 :中国化学快报(英文版) | 被引量 : 0次 | 上传用户:as55059550
下载到本地 , 更方便阅读
声明 : 本文档内容版权归属内容提供方 , 如果您对本文有版权争议 , 可与客服联系进行内容授权或下架
论文部分内容阅读
The disinfection of waterborne pathogens from drinking water is extremely important for human health.Although countless efforts have been devoted for drinking water inactivation,challenges still exist in terms of relative high energy consumption and complicated to implement and maintain.Here,silver nanoparticles anchoring wood carbon (Ag NPs/WC) membrane is developed as cost-effective,high flux,scalable filter for highly efficient electric field disinfection of water.Under electric field of 4 V voltage,the designed membrane achieved more than 5 log (99.999%) disinfection performance for different model bacteria,including Escherichia coli (E.coii),Enterococcus faecalis (E.faecalis),Salmonella enterica serovar Typhimirium (S.Typhimurium) and Bacillus subtilis (B.subtilis) with a high flux of 3.8 × 103 L m-2h-1,extremely low energy consumption of 2J L-1 m-2 and fantastic durability (7 days).The high disinfection performance of Ag NPs/WC membrane is attributed to the synergistic disinfection of carbon nanofibrils,Ag nanoparticles as well as the low tortuous structure of the channels in wood carbon.The Ag NPs/WC membrane presents a promising strategy for point-of-use drinking water electric field disinfection treatment.
其他文献
Low-efficiency charge transfer is a critical factor to limit the photocatalytic H2 evolution activity of semiconductor photocatalysts.The interface design is a promising approach to achieve high charge-transfer efficiency for photocatalysts.Herein,a new 2
Metal-organic frameworks (MOFs) have a regular porous structure and high porosity,which make them ideal electrode materials for supercapacitors.However,their capacitance performance is greatly limited by their poor conductivity.In this study,a multi-compo
To prevent polysulfides from dissolution into electrolyte,we propose a novel and simple approach to nitrogen-doped carbon foams which contain hierarchically porous structure and are decorated with zinc nanodots through one-pot carbonization and activation
We have developed a facile strategy to fabricate model multicolor hydrogels via a straightforward mixing process of poly acrylonitrile-grafted methacrylamide (PANMAM),polymethacrylic acid (PMAA) and doped lanthanide (Eu/Tb) and zinc ions to form the inter
The silicon-based materials are promising candidates for lithium-ion batteries owing to their high energy density.However,achieving long lifespan under realistic conditions remains a challenge because of the volume expansion and low conductivity.In this w
Ammonia (NH3) is considered an attractive candidate as a clean,highly efficient energy carrier.The electrocatalytic nitrogen reduction reaction (NRR) can reduce energy input and carbon footprint;therefore,rational design of effective electrocatalysts is e
In this paper,a novel BC3N2 monolayer has been found with a graphene-like structure using the developed particle swarm optimization algorithm in combination with ab initio calculations.The predicted structure meets the thermodynamical,dynamical,and mechan
Trimethoprim (TMP) is a typical antibiotic to treat infectious disease,which is among the most commonly detected antibacterial agents in natural waters and municipal wastewaters.In the present study,the impacts of dissolved oxygen (DO) on the oxidation ef
In this study,Si-doped ferrihydrite (Si-Fh) was successfully synthesized by a simple coprecipitation method for removal of heavy metals in water.Subsequently,the physicochemical properties of Si-Fh before and after adsorption were further studied using se
Accurate detection of hydrogen sulfide (H2S) is of great significance for environmental monitoring and protection.We propose a colorimetric method for the detection of H2S by the use of mixed-node Cu-Fe metal organic frameworks (Cu-Fe MOFs) as highly effi