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Arc Spray Nanoparticle Synthesis System (ASNSS) has been used to prepare the silver nanofluids in this study. The metal electrodes under the electrical discharge will melt and evaporate rapidly and condense to form the nanoparticles in the dielectric fluid at lower temperature and produce the suspended nanoparticle fluid. Thus, the mechanism of the ASNSS process is superheating the electrodes by plasma to form metallic nuclei and supercooling these nuclei by dielectric liquid to produce nanofluid. This study considers the different controlling parameters such as discharge current,discharge voltage, pulse-duration time, electrode diameter, and the temperature of dielectric liquid. The optimally operated parameters can be obtained to produce the finer particle size in nanofluid. The results indicate the silver electrodes in alcohol fluid will produce the spherical nanosilver particles. The mean particle size of silver in different dielectric liquid temperatures of-40, -20, 0, and 10℃ is about13.4, 15.8, 17.5, and 21.6 nm, respectively. This indicates that the well suspended fluid can be obtained by controlling the lower dielectric fluid temperature.