Electrolytic cell engineering and device optimization for electrosynthesis of e-biofuels via co-valo

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Utilizing CO2 in an electro-chemical process and synthesizing value-added chemicals are amongst the few viable and scalable pathways in carbon capture and utilization technologies.CO2 electro-reduction is also counted as one of the main options entailing less fossil fuel consumption and as a future electrical energy storage strategy.The current study aims at developing a new electrochemical platform to produce low-carbon e-biofuel through multifunctional electrosynthesis and integrated covalorisation of biomass feedstocks with captured CO2.In this approach,CO2 is reduced at the cathode to produce drop-in fuels (e.g.,methanol) while value-added chemicals (e.g.,selective oxidation of alcohols,aldehydes,carboxylic acids and amines/amides) are produced at the anode.In this work,a numerical model of a continuous-flow design considering various anodic and cathodic reactions was built to determine the most techno-economically feasible configurations from the aspects of energy efficiency,environment impact and economical values.The reactor design was then optimized via parametric analysis.
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