CORRELATION OF ALKALINITY WITH AROMATIZATION SELECTIVITY OF C_6 PARAFFIN OVER Pt/ML(M=Li,Na,K AND Rb

来源 :Journal of Natural Gas Chemistry | 被引量 : 0次 | 上传用户:fpkneo
下载到本地 , 更方便阅读
声明 : 本文档内容版权归属内容提供方 , 如果您对本文有版权争议 , 可与客服联系进行内容授权或下架
论文部分内容阅读
The effect of alkaline metals such as I,i, Na, K and Rb on the aromatization of n-C6, paraffin over Pt/ML zeolite catalyst was studied. It was shown that the alkaline cations, especially the Rb with strong basicitv and larger radius, lead Pt particles to disperse well on the surface of L zeolite. A stronger basicity of the modifying cation resulted in higher activity and selectivity to aromatization of n-C6. It is argued that the alkali cations affected the electronic slate of P1. leading to Ptδ-. which caused a decrease of dehvdrogenation activity and an increase of the selectivity to aromatization. The effect of alkaline metals such as I, i, Na, K and Rb on the aromatization of n-C6, paraffin over Pt / ML zeolite catalyst was studied. It was shown that the alkaline cations, especially the Rb with strong basicitv and larger radius, lead Pt particles to disperse well on the surface of L zeolite. A stronger basicity of the modifying cation resulted in higher activity and selectivity to aromatization of n-C6. It is argued that the alkali cations affected the electronic slate of P1. to Ptδ- which caused a decrease of dehvdrogenation activity and an increase of the selectivity to aromatization.
其他文献
一九九八年六月六日,有一支12人组成的审计小组悄然上路,直奔兴山,在这支队伍中,有一位年过半百的长者,他就是兴山粮食审计工作的副总指挥王合钧同志。熟悉的人都知道,在履
我院1980~1982年收治的肝炎患者中,在排除其它病毒感染或药物等因素后,有14例患者并发皮肤损害,占1:66%。出现皮损之后,病情好转,均痊愈出院。提示病毒性各型黄疸性肝炎皮肤损
编者按:近年来,在纪录片的创作实践中,出现了虚构手法的运用,而电视纪实作为一种手段,也被广泛应用到各类电视节目的创作中。面对混杂不清的现实,围绕电视纪实的本质,学界展
自公元前1000年初以来就未曾中断的文本记录,作为文化和政治的正统来源享有很高的威望,字里行间似乎容纳了中国早期历史进程的清晰画卷。首先出现的是许多独特的文化英雄般的
两个根本性转变的历史选择刘国光中国发展社会主义经济,至今已经历近半个世纪。在这段时期中,我们工作重点是如何将丧失了近百年发展机遇的时间抢回来,如何使生活在占世界7%土地上
刘××,男,42岁,工人。 1974年6月15日上午10时许,因腹痛腹泻来站门诊,诊断为肠炎,予合霉素0.5克每日4次,颠茄片8毫克每日3次口服。病人当日下午3时许服合霉素0.25克,服后2
本实验研究了脑源性神经营养因子(brain derived neurotrophic factor,BDNF),神经生长因子(nerve growth factor,NGF)和神经营养因子-3(neurotrophin-3,NT-3)的mRNA和蛋白在
本院收治一例脑垂体嗜酸性腺瘤引起肢端肥大症女病人,容貌、性格均明显呈男性化改变,同时伴发精神障碍,因临床较罕见,现报道如下:高××,女,44岁,社员,1980年2月6日入院。病
建立了一种测定UO_2-Gd_2O_3烧结芯块氧与金属原子比(简称O/M比)的新方法——分光光度法。以浓磷酸为溶剂,U~(6+)和U~(4+)离子的特征吸收波长分别确定在310nm和544nm。U~(6+