Ultrafast Quasiparticle Dynamics and Electron-Phonon Coupling in(Li0.84Fe0.16)OHFe0.98Se

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Distinctive superconducting behaviors between bulk and monolayer FeSe make it challenging to obtain a unified picture of all FeSe-based superconductors.We investigate the ultrafast quasiparticle (QP) dynamics of an intercalated superconductor (Li1-xFex)OHFe1-ySe,which is a bulk crystal but shares a similar electronic structure with single-layer FeSe on SrTiO3.We obtain the electron-phonon coupling (EPC) constant λA1g (0.22 ± 0.04),which well bridges that of bulk FeSe crystal and single-layer FeSe on SrTiO3.Significantly,we find that such a positive correlation between λA1g and superconducting Tc holds among all known FeSe-based superconductors,even in line with reported FeAs-based superconductors.Our observation indicates possible universal role of EPC in the superconductivity of all known categories of iron-based superconductors,which is a critical step towards achieving a unified superconducting mechanism for all iron-based superconductors.
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