Trace Determination of Zirconium(Ⅳ) by Anodic Adsorptive Voltammetry at a Carbon Paste Electrode

来源 :Chinese Chemical Letters | 被引量 : 0次 | 上传用户:zhongqiwen
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A new sensitive adsorptive voltammetric method was described for the determination of zirconium at a carbon paste electrode (CPE) in the presence of alizarin complexone (ALC). Optimal analytical conditions are: 1.0?0-6 or 5.0?0-7 mol/L ALC, 0. 20 mol/L HAC-NaAc (pH 4.3), accumulation for 60 s at 0 V (vs. SCE), and linear scanning from 0 V to 1.0 V at 250 mV/s. The peak potential of the complex is at 0.81 V. By using a model JP-303 polarographic analyzer, 2.0?0-10 mol/L (S/N=3) zirconium can be detected with a 90 s accumulation, when the 2nd-order derivative linear sweep technique is used, and the linear range is 6.0?0-10-2.0?0-8 mol/L (5.0?0-7 mol/L ALC) and 2.0?0-8-2.0?0-7 mol/L (1.0?0-6 mol/L ALC), respectively. The developed method was applied to the determination of trace zirconium in the ore samples with satisfactory results. A new sensitive adsorptive voltammetric method was described for the determination of zirconium at a carbon paste electrode (CPE) in the presence of alizarin complexone (ALC). Optimal analytical conditions are: 1.0? 0-6 or 5.0? 0-7 mol / L ALC, 0. 20 mol / L HAC-NaAc (pH 4.3), the accumulation for 60 s at 0 V (vs. SCE), and linear scanning from 0 V to 1.0 V at 250 mV / s. The peak potential of the complex is at 0.81 V. By using a model JP-303 polarographic analyzer, 2.0? 0-10 mol / L (S / N = 3) zirconium can be detected with a 90 accumulation, when the 2nd- 0-10-2.0? 0-8 mol / L (5.0? 0-7 mol / L ALC) and 2.0? 0-8-2.0? 0-7 mol / L (1.0? 0-6 mol / L ALC), respectively. The developed method was applied to the determination of trace zirconium in the ore samples with satisfactory results.
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