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With fast developing in nanoscience and nanotechnology, it has been a great challenge on how to synthesize high quality nanoscale building blocks in macroscopic-scale and assembly them into macroscopic assemblies with diverse functions.Through systematical study in past several years, we have demonstrated that the ultrathin tellurium nanowires can be employed as a versatile template for templating synthesis of a series of high-quality 1 D nanostructures by taking advantages of the unique features of TeNWs, i.e., large-scale synthesis, high processability and high reactivity.