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Ceramic electrolytes (CEs) and solid polymer electrolytes (SPEs) are considered to be effective methods to suppress the growth of lithium dendrites.But the inferior wettabilityof CEs and the low ionic conductivity of SPEs limit their applications.Zhang and colleagues report in Advanced Materials that flexible ceramic/polymer hybrid solid electrolyte-prepared by in situ coupling reaction-has great promise for high-performance Li metal batteries (LMBs).