Precursors and potential sources of ground-level ozone in suburban Shanghai

来源 :环境科学与工程前沿 | 被引量 : 0次 | 上传用户:ssskstar
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A high level of ozone(O3)is frequently observed in the suburbs of Shanghai,the reason for this high level remains unclear.To obtain a detailed insight on the high level of O3 during summer in Shanghai,O3 and its precursors were measured at a suburban site in Shanghai from July 1,2016 to July 31,2016.Using the Hybrid Single-Particle Lagrangian Integrated Trajectory(HYSPLIT)model and concentration weighted trajectories(CWT),we found that Zhejiang province was the main potential source of O3 in suburban Shanghai.When the sampling site was controlled by south-western winds exceeding 2 m/s,the O3-rich air masses from upwind regions(such as Zhejiang province)could be transported to the suburban Shanghai.The propylene-equivalent concentration(PEC)and ozone formation potential(OFP)were further calculated for each VOC species,and the results suggested that propylene,(m+p)-xylene,and toluene played dominant roles in O3 formation.The Ozone Isopleth Plotting Research(OZIPR)model was used to reveal the impact of O3 precursors on O3 formation,and 4 base-cases were selected to adjust the model simulation.An average disparity of 18.20%was achieved between the simulated and observed O3 concentrations.The O3 isopleth diagram illustrated that O3 formation in July 2016 was in VOC-sensitive regime,although the VOC/NOx ratio was greater than 20.By introducing sensitivity(S),a sensitivity analysis was performed for O3 formation.We found that O3 formation was sensitive to propylene,(m+p)-xylene,o-xylene and toluene.The results provide theoretical support for O3 pollution treatment in Shanghai.
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